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<br />.,.,,-' <br /> <br />. -"-~...-~ <br /> <br />.--.--- <br /> <br />1 ... H <br /> <br />'EV/J.uAT1I)~~ ('Ir r:COLOi.:tCAt EFFE.CTS DF SILv'ER IOiJTD~. SEEnING AGENT).I <br />? I <;,-,~:o' 1 <br />;)c"inlllJ 0\. Klein:':' and RiC'hilrd ,'L <br /> <br />Accumulatio; oi silver iodide from <br />weather modification ~ill result 1n nc <br />overt toxicity effects, but may re$1I1: <br />in a slight d~lay in biological <br />pro.cesses. <br /> <br />11 In Steinhoff, H.~J., ",nd J.D. rves (F.ds). 1976. Ecolo!tical impac.ts of snowpack <br />Mountains. Colorado. San Juan Ecolo~y Project. fl.nal Report. Colorado State <br />1/ Present address; Dept. of HicrobioloF!),. CcloraJo State liI1:\v., Ft. ColUns. Co. <br /> <br />ABSTRACT <br /> <br />The possible effectS of silver iodide seeding agent <br />accu~ulation in surface soil& of the San Juan area <br />were investigated by use of laboratory studies in- <br />volv:1ng Arthrobaccer - silver interactions. treatment <br />of soils with varied forms alld level!! of silver, by <br />examination of silver gradients surrounding seeding <br />genetator sites. and by use of treatment plots in <br />spruce, aspen. and subalpine meadow communities <br />located in the San Juan snoV augmentation area. Lab- <br />oratory studies have shown that on a short-term basis" <br />silver iodide or seeding generator burn mixtures at <br />hi~her than field concentration show only slight <br />effects on microbial growth or enzyme function. while <br />free silver ions, even at part-per-billion levels. <br />can eaus~marked chanses in microbial activities. <br />TheSe effects were -le*sened in the presence of sailor <br />complexing.ions. HOwever, under field conditions on <br />a 3 year basis, Bilve~ iodide appears to have a great- <br />er potential fer altering pail decomposer ,functions <br />than silver from".sUver ion. The presence of sUver <br />from silver iodide - todium iodide complexes, again at <br />higher than background levels. in the San Juan target <br />area led to a gradual increase in soil organic matter <br />content in spruce.and _aspen surface solIs. No such <br />incr~a8e was obaerved in the 8ubalpine meadow plot. <br />Silver from silver nitrate tended to concentrate more <br />in upper plant portions than silver from silver iodide, <br />although silve~ from silver iodide was more closely <br />associated with the plant roots. These effects were <br />only observed 'using silver levels lo-lOOX expected <br />field accumulation levels. Based on the available <br />literature and experiments carried out to date, the <br />accumulation of silver iodide seedin& agent does not <br />appear to present an ecological threat. although con- <br />tinual monitoring of test systems should be carried <br />out to extend the time period over which this conclu- <br />sion can be tested. <br /> <br />OBJECTIVES AND HYPOTHESES <br /> <br />1. <br /> <br />To monitor soil microbial activities in the San <br />Juan area, to determine if possible silver accre- <br />tion is influencing soil microbial processes. <br />To analYze treatment plot soils to which various <br />silver addjtons have been made in aspen, spruce, <br />and grass communities. <br />To measure microbial responses to silver gradients <br />present 1n the vicinity of the pagoas Springs gen- <br />~rator s1te No. 25. and the Emerald Mountain site. <br />To determine the existence ot possible sub-lethal <br />effects 01: varlee SlJ.ver J.eve.Ui ana {u{m~ un <br />microbial processes. including ettects on mlcrOOl- <br />al viability and capabilit1es to ttanstorm su~ <br />strates requiring enzymatlc adapcatIOn ana enefgy- <br />p'roduction processes. <br />To determine if soil microbes are capable of <br />transforming silver present as silver 10d~de to <br />additional silver forms. and to determine physio- . <br />logical mechanisms which may result in silver <br />transtormac10ns. <br />To determine if assay procedures Cor vnricd s11ve~ <br />Corms in soil can be developed. <br /> <br />2. <br /> <br />), <br /> <br />4, <br /> <br />5, <br /> <br />6, <br /> <br />These objectives have <br />hypotheses: <br /> <br />.'~-'Hypochesis L <br /> <br />been summarized in a series of <br /> <br />'" <br /> <br />: Hypothesis II. Laboratory studies can give an indic,'l- <br />tlon of the degree of possible dim1n- <br />uation of microbial activity which <br />might result froIll silver ac:cumul...tion. <br />Ill. Soil bacteria can cause a ~hang( in <br />silver iodide to forms more e~s:\ly <br />taken up by plants. This mpdification <br />of silver form may make it necessary <br />to carry out experiments under field- <br />related conditions as much as possible. <br /> <br />-R,,~ly,..s S~c'f,'onj D';';tf'e.j.-: <br /> <br />i <br /> <br />i <br />: Hypothesis <br /> <br />,UHMARY <br /> <br />Based on work carried out on the possible ecolof,icilJ. <br />effects of silver iodide seeding agent accumulation in i <br />salls of the San Juan area. the following conclusions <br />CAn be drawn: <br /> <br />2. <br /> <br />The accumulation of silver iodide nucleatin~ agent~ <br />presents lJo_.ov~rt-dan&er to humans, pla.nts or .ani- <br />I mals. based on available literature and work car- <br />ried out under this studv for a J \-'ear oer1od. -- <br />Silver 10n can cause decreased grovch and enzYme <br />-induct 10n 1n a soil Archrobacter sDecies aL1=.l.o. <br />ppb free silver ion. The effect observed is depen- <br />dent on other anions and cations preserit. Soil <br />decreases the activity of free silver ions. <br />Silver from silver iodide or burn mixtures does <br />not show such ettects on mlcrobla~ grow~n or en- <br />zymatic activity. Generally 10-IUU ppm ot AgI <br />torm silver 1s required to observe effects on <br />growth, VIability. and enzyme induct1on. <br />Free silver ion trom ~ilver iodide dissociation at <br />5~6 ppb can cause'observable effects on micro_ <br />organisms. To achieve this silver level <br />100-200 ppm of silvei as silver iodide a~e re- <br />quired. <br />Microorganisms can cause reduction of free silver <br />ion or silver iodide to metallic silver. Amine- <br />type materials may be responsible for this reduc- <br />tion. <br />Silver iodide added at 1000 ppm shows no immediate <br />effects on soil respiration processes. <br />Attempts to establish respiration indices for test <br />soils across the impact area vere not successful <br />due to short-term varrability of soil. moisture and <br />temperature. <br />Silver accumulation in the vicinity of two seeding <br />enerator sites did not cause decreases 1n m1cro <br />bial respiration. Silver tended to accumu ate and <br />remain 1n the surl:ace Boil zone In Sp~~e ot ex- <br />tended vater percolation through the zone. <br />A subalpine meadow test plot installed for ) years <br />USing silver iod1de and silver n~trate at I, lU, <br />100 ppm surl:ace soil levels did not show changes <br />in decomposer functions which could be relate~to <br />this treatment. - -. <br />Silver from silver iodide moved to upper plant por- <br />tions.to a lesser extent than silver from silver <br />nitrate. <br />Silver from silver iodide was more closely associ- <br />ated with plant roots than silver from silver ion. <br />After 3 years, silver from these tvo differing <br />original forms have not equilibrated to forms <br />which will give similar activities. <br />In spruce and aspen plots, imposition with silver <br />iodide tends to be related to increased organic <br />matter retention in the test systems. No such <br />relationships were observed with equivalent treat- <br />ments using silver from silver nitrate (silver <br />ion) . <br /> <br />1. <br /> <br />), <br /> <br />4, <br /> <br />5, <br /> <br />6, <br /> <br />], <br /> <br />B, <br /> <br />9, <br /> <br />10, <br /> <br />11. <br /> <br />12, <br /> <br />, <br />, <br />\ 13. <br />, ! <br /> <br />augmentation <br />Volv. Publ.. <br />8052), ' <br /> <br />in the San Juan <br />Fort Collins. <br />