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<br />APRIL 1995 <br /> <br />839 <br /> <br />1500 <br /> <br />1500 <br /> <br />MEYERS ET AL. <br /> <br />1500 <br /> <br />1500 <br /> <br /> <br />1000 <br /> <br />i a <br /> <br />. . . . <br />..........,............,...... .....v............,......... <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />. . . . <br />.. . <br />.. . <br />.. . <br />.. . <br />.. . <br />.. . <br />.. . <br />.. . <br />. . . . <br />. . . . <br />. . . . <br />..........f"............,............':'..........I.......... <br />. . . . <br />. . . . <br />. . . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br />. . . <br /> <br />500 <br /> <br />1000 <br /> <br />.............;...........\ .1..............1............ <br />I ~i\ i <br />! " l <br />l ! <br />i \ ! <br />! ! <br />.............J............... .............~............. <br />: : <br /> <br /> <br />I i I <br /> <br />~ <br />~ <br /> <br />Ql <br />E <br />i= <br />500 <br /> <br /> <br />o <br />-1 <br />1500 <br /> <br />-.5 0 .5 <br />100(Sw-l) (~) <br /> <br />o <br />-10 -9 -8 -7 -6 -5 <br />Temp (,C) <br /> <br />1500 <br /> <br />~ <br /> <br />I <br /> <br />!. I I! <br /> <br />.......f..........I.........~.....j...~......i. }....... <br />I I I! I : I <br />I ! I II : I <br />i i i i i : i <br />.......t..........t.........I......j...t.....!. i........ <br />! . ! I! :! <br />! I i I : I <br />! !j j : j <br />o <br />.1 .3 1 3 10 130 100 <br />Cond-Frz. (L- ) <br /> <br />~T <br />-r- <br /> <br />e <br /> <br />I <br />! I <br /> <br />1000 rri <br />~rn! <br /> <br />o <br />.1 .3 1 3 19 30 100 <br />Depos. (L - ) <br /> <br />1000 <br /> <br />Ql <br />E <br />i= <br /> <br />500 <br /> <br />b <br /> <br />d <br /> <br />c <br /> <br />1000 <br /> <br />\ ,. i <br /> <br />..............'+\..............-t.................. <br />r i i <br />! i I <br /> <br />..................4...... .............~.................. <br /> <br /> <br />1000 <br /> <br />500 <br /> <br />500 <br /> <br />I I ~'I I <br />i i i i <br />! ! ! ! <br />i !! <br />: :: <br /> <br />o <br />o <br /> <br />o <br />o <br /> <br />2 4 6 8 10 <br />Drop Radius ~m) <br /> <br />100 200. 300 <br />Drop Cone. (em-) <br /> <br />1500 <br /> <br />1500 <br /> <br /> <br />h <br /> <br />f <br /> <br />g <br /> <br />.. .r <br />1000 .....-r........t.........t.....t..7i...... <br />i i i i.l i <br />I I I Jt I <br />500 .......!..........l.........!....../L...." : ....... <br />! i i / i,' j <br />i i X ),' i <br />! i': I: ! <br />! V V! ! <br />)/i./ i i <br />o <br />.1 .3 1 3 10 ~O 100 <br />Contaet-Frz. (L-) <br /> <br />1000 <br /> <br />, ., Ii. i <br /> <br />.....l/"l/ ...t.........r......l...... <br />JilJJJ- <br /> <br />. . . . . <br />: : : : <br />. . . . <br />: : : : <br />1 ! ! ! <br />! ! ! ! <br />. . . . <br />: : : : <br />. . . . <br />1 ! ! ! <br />. . . . <br />. . . . <br />1 ! ! ! <br />! ! ! i <br />: : : : <br /> <br />500 <br /> <br /> <br />o <br />.1 .3 1 3 10 391 100 <br />Immersion-Frz. (L ) <br /> <br />FIG. 3. Parcel model simulation temporal profiles of (a) temperature, (b) percent water supersaturation, (c) droplet concentration, (d) <br />average droplet radius, and (e)-(h) cumulative ice crystal concentrations nucleated by different ice-formation modes. Dashed curves are for <br />the presumed aircraft generator particle size distribution. The dash-dot curves presume the size distribution given by DeMott et al. (1983) <br />for a ground-based generator. The solid curves are from the parameterized equations (aircraft generator PSD). <br /> <br />The detailed equations from DeMott ( 1994) were used <br />in these simulations. It is seen that the size distribution <br />can be quite important to the realized effect of seeding <br />on ice crystal concentrations. A factor of 3 decrease in <br />concentrations was noted when the size distribution <br />measured from a ground generator was used instead <br />of the typical airborne generator distribution. The <br />somewhat lower ice nucleus activity of the smaller <br />aerosols produced qy aircraft units was more than <br />compensated for by the increased numbers of smaller <br />particles. The airborne generator size distribution was <br />deemed most appropriate for use in the mesoscale sim- <br />ulation. Figure 3 also demonstrates the excellent per- <br />formance of the parameterized descriptions of ice-for- <br />mation processes. The simulation results using the pa- <br />rameterized equations developed for use in the <br />mesoscale model are indicated by the solid curves in <br />Fig. 3. These results are directly comparable to the <br />dashed curves (detailed equations, aircraft generator <br />PSD). Only a very slight tendency for the parameter- <br />ization to overestimate ice formation was found. <br /> <br />Figure 3 also demonstrates that the initial concen- <br />trations of ice nucleated when AgI-AgCI aerosols are <br />released directly into a wintertime orographic cloud <br />will come primarily from deposition and condensation- <br />freezing events and will therefore strongly depend on <br />the ambient humidity or any higher supersaturation <br />potentially generated during combustion (Finnegan <br />and Pitter 1988). For the initial conditions specified, <br />deposition and condensation freezing contribute nearly <br />30 L -I, representing approximately 0.02% of the total <br />aerosol almost instantly for the aircraft generator PSD. <br />Condensation freezing was less important at later times <br />despite the decrease in temperature because water su- <br />persaturation decreased to near zero. Deposition con- <br />tinued to generate significant numbers of ice crystals <br />as the temperature decreased and ice supersaturation <br />increased. Contact freezing was predicted to be a minor <br />player for the first several minutes after seeding because <br />collection rates are slow in the orographic cloud and <br />nucleation efficiencies are lower at warmer tempera- <br />tures. This mechanism began to dominate ice forma- <br />