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<br />. <br /> <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br /> <br />where Nid (1-1) is the number of pristine ice crystals predicted due to deposition- <br /> <br />condensation freezing, a = -0.639, b = 0.1296, and S; is ice saturation ratio. In addition, <br /> <br />Young's estimates of contact nuclei concentration were replaced with estimates from <br />laboratory experiments by Vali (1974, 1976), Cooper (1980), and Deshler (1982). The <br />formula for contact nucleation takes the form, <br />N;c = exp[a + b(273.15 - I:)] <br /> <br />where a = -2.80 and b = 0.262, is used [units of N. are inverse liters (1-1)]. In version <br />IC <br />4.3 we have added an option to predict the vertical and horizontal transport of ice- <br />forming nuclei (IFN). Thus in cases where soundings of IFN are available we now have <br />the capability of predicting the vertical mixing and transport of IFN from high to low <br />concentration regions and vice versa. This also permits the addition of an IFN source <br />such as ground-based generators to simulate cloud seeding. <br /> <br />The secondary ice particle production model in RAMS is based on Mossop (1978) in <br />which he derived the empirical relation: <br />Ni = c N24 (N'3)m (2) <br />where N1 is the number of ice particles produced per second, N24 is the number of cloud <br />droplets larger than 24 microns in diameter that are collected by ice each second, N13 is <br />the number of cloud droplets smaller than 13 microns in diameter that are collected by ice <br />each second, m is an exponent equal to 0.93, and c is a constant of proportionality. This <br />relationship was derived from a laboratory apparatus in which supercooled cloud droplets <br />were collected on a glass rod, and experiments were conducted for a wide range of <br />droplet concentrations, leading to many different values of N24 and NI3' <br /> <br />We re-interpreted the empirical results ofMossop by accounting for the cross-sectional <br />area of the glass rod, which was 5.4 cm2. In RAMS, we thus compute N24 and NI3 per <br />5.4 cm2 of cross sectional area of ice particles that collect cloud water, and apply the <br />above formula. In MKS units, the formula is: <br /> <br />Nj = 9.1e-l0 x B x N_24 X (N13}93 (3) <br /> <br />where B increases linearly from 0 to I as ice temperature T increases from -8 C to -5 C, <br />B decreases linearly from 1 to 0 as T increases from -5 C to -3 C, and B is zero at other <br />ice temperatures. <br /> <br />At colder temperatures such as found in cirrus clouds, primary nucleation by <br />homogeneous freezing of supercooled cloud drops and haze particles was introduced <br />(DeMott et aI., 1994). Ice is categorized in RAMS into pristine ice, which is pure vapor- <br />grown crystals, and snow, which is larger vapor-grown crystals and crystals that undergo <br />moderate riming (Harrington et aI., 1995). Aggregates remain as a separate category, as <br />well as low-density graupel particles. Hail is an additional category that represents high- <br />density frozen particles such as frozen raindrops and hailstones. <br /> <br />II-IO <br />