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<br />ROCKY ]FLATS SOIL PLUTONIUM'"'240 SURVEYS FROM 1970 TO 1991 <br />' Higher resolution sampling and point data with accurate location coordinates sufficient to draw <br />contours could highlight the area of concern more accurately. Probabilistic models and contours <br />to definitively predict concentrations as a function of distance and direction to isolate the <br />boundaries of those areas, respectively, are possible with the proper data. The sampling plan <br />design that obtained the results in this report was not developed for such a level of analysis. <br />The spati;tl distribution evident in the graphical and GIS analysis are sufficient to cleazly show <br />that plutonium79z"0 data is not randomly distributed around Rocky Flats. The spatial <br />distribution of plutonium is dependent on distance, direction, wind speed, wind direction, <br />particle sizes, etc. and is tied directly to one or more past events. These events include winds <br />either at the time of excavation and covering of the 903 Pad, 1967-1969 and or winds after the <br />' 903 Pad was initially capped. Given the decrease in plutonium concentrations in an eastern <br />direction, plutonium139+2°0 correlated to particulate sizes may be a strong indicator and <br />mechanism to base plutonium79240 concentrations as a function of distance and direction from <br />the 903 Pad. This could be a basis to explain the reduction in plutonium79zd0 with distance from <br />the 903 Pad. If the plutonium79+2"0 distribution was primarily caused by one source, then such a <br />relationship would be easier to identify. The CDH data, though not quantified, strongly indicates <br />that the 9~)3 Pad is the primary source of plutonium contamination. <br />A mathematical relationship tied to distance would need to consider particle sizes and associated <br />plutoniutri79370 concentrations. Part of the model would be an expression of the mechanistic <br />process that resulted in the release of plutonium23'210. Wind speed and wind direction would be <br />additional variables to perform sensitivity analysis to isolate conditions that occurred during the <br />release from the 903 Pad. The CDH Health Studies on Rocky Flats are developing this portion <br />of the model. The other part of the model would be an explanation of plutonium concentrations <br />now press:nt in the soils. Contours would be drawn from this model and compared to the <br />observation. Statistical analysis would be used to compare the accuracy of the observations to <br />model results. The later part of the model is the subject of DOE RFURI work under the <br />Interagency Agreement IAG with DOE, CDH and EPA. (USDOEa; USDOEb) <br /> <br />l <br />1 <br /> <br /> 23 <br /> <br />