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<br />GR01....nwA11-:R RES/l1FSCE n\/E. ,-t\O RI'OHRCE n~IIPHUTl"RE E\TIIH11--S OF 11110 DEWEl< ASD .4RAP.-tilOf AQf1H.kl, DE..\l"f.R 8.4..\"/.\, COWR.'iDO <br /> <br />Rl"Cha~e Temperature <br /> <br />Tht' tCffipt'r.lturt" of rcchaT'Ring groundwatt"r, :10 approxi- <br />mation of mean-annual air tempt'r.uure, can he estimJ.t...d <br />from con("t"ntrJ,tion:-. of atmo~pheric nook 1l:1St".;. diS-.'iol\"(~d <br />in groundw:Ul;'f using lht" general lempt'"ratllR"~as soluhil- <br />ity rd:ltionship, Henry's Liw (e.g., ~tute el al., 1992; <br />At"Sl.:hhadl-Henig t"1 aI., 1999). TIll' concentr.ltIons of int'rt <br />Ra~s in gmundwater rt"sull from thl.:' lempt"r,llure- and <br />pressure (de\';Hion)- ut:pcndent equihhration of w:Uer with <br />the atmosphere, plus IhlO" addition of eXct's.'i air arising <br />from dissolution of entr.Jined air huhhks h<:low the walef <br />tahle (~tu!e and Schlosser, 200m, TIll.' excess air may be <br />fr:Il..'1ionah."d due to partial dissolution or r""-t.'quilihr::uion of <br />th.... gas (At'schhach-Hertig ...'1 :11.. 1999), <br />\'ari:lIion in pak"Olempt'"ratllfes t'stim:ued from conn:n- <br />trations of nohle WISl..'S su~...'st.... a templ..'r.\Iure suppression <br />rangin~ from ;-9'C during the last gbci:11 period <br />(Aeschbach-Hertig et al.. 10(0). :Sohle ga:-. tt"lllpcr.ltures in <br />the south-centr31 and southwestern U.S, dllfin~ the \;I~t <br />glacial period were approximatdr :;'C cookr th;1O <br />Holon'ne tell1per.nur....~ (Stule t-'t ;II., 1991; Clark d al.. <br />199K), consistent with other c..timalt.'s of l'ontinl..'ntal tem- <br />per.Hure change and local gbcial-clinutt" recunstmctions <br />(.\1uhs et a!., 1(99). <br /> <br />METHODS <br /> <br />Samplin~ <br /> <br />Six samples wefe l'ollectnl from kx:;lliun.'i that lie along <br />a tr.mseCl p;lr:illld to the pre...urneu mOlkrn ,!o:fuundw3tl:'r <br />now palh heginnin~ ne;lr tilt' sOllth...'rn oulcrop of the <br />~Iquifer:'o (Fi~, 1), 111t' ,~Jmple.~ were uJlleckd from ground- <br />watt'r of the Ar.:lpaho... and Denver aquifer;, nt'ar P:lfker. <br />Colorado during the ~pring of 2001 ;lnd ne:lr Aurora anu <br />[xlOala (n..."ar Colorado ~prings), Colur.Jdo durinll the <br />~pring of 2(X~5 I Tahle I). One,liwr \Vatl..'r :'oampiL's Wt're <br />analyzlO"d for dh.~olved inorganic ...';\fl-xm (DIC) i."-OlOpes hy <br />atomic mas...-sp...'cuomcuy al Ikt:1 :\nal}"tical LIhs, Ih:;,ults <br />of DiC :Illaly~i;, .Ire fl..'pOI"tl'd in pcf('....nt mOl!...'rn Glrhon <br />(POlO for HC and delta l3-culxlO per mil \l-'DB IOl:lC '%0) <br />for rdati\"(~ UC/l~C. S~lmpks for di:'o~oln.d !o(.IS analy~es <br />w...'re collected follo\ving Ihc prolOcol outlmed hy :-o.l.:mning <br />et a!. (2()()3) :md were an:llyzt--d hy the :'\ohk- Gas Llhora- <br />{{)IT at the Univt'rslty of ('tah for 2li.,\~ .i~02' 211:\'e. lilAr, <br />l'>IKr. .~Ht' anJ\He. Results of the Ji......olv'ed g.ls ;lOalysis arc <br />r""p<lrted in mol.lr-fraction (unit-less) and precision of mea- <br />surement.'i i.-; a f...,\\ iX'rn:nL Additional fidd mea:-.tIfemenl<, <br />of fempt'"ratun~ IT) ;lml tot:lI Jissolwd gas pn5Sure (PllX,) <br />of the groundwater were made. :\ lktailcd dcsLriplion of <br />the samplin,g prol..'edure :Ind ;lIlaly"i" may IX' found in <br />:'\:o\'otny (2rxH~. <br /> <br />A 0 <br /> <br />20 <br /> <br />i:L... <br /> <br />, " <br /> <br /> <br />LEGEND <br />o SampleLocebOf1 <br />o AtlurferOulcrop <br />UrbanAloa <br /> <br />Pot.ntrom.tric: Surtac:.: <br />Incremel'1lsofl00!'l1l'om <br />hi9" (dal'k) 10 low (l9ht) <br />surfaceCO'llOU' <br /> <br />figure 1, General locations of groundwatPf samples with 197B <br />pOlentiOmetric surface of Arapahoe aquifer (Robson, 1987) for <br />reference. <br /> <br />Carbon-14 Activity Dilution and Determination of <br />Residence Time <br /> <br />Additional sources of carl-xm exist in most ;Iquifcrs and <br />("'.In t:au'\t" dilUlion of thc !-IC acth-ilY. nu:rd(m:~. a corret:- <br />[ion for tht" interal'1ion of thest.' SOtlfCI:'S with grollndwatl'r <br />wa~ :Jpplk'd prior 10 Ihe cakubtion of resid....nn: time. Cor- <br />rection mt'th(xb in\"olving mas..'i-habnce of oC/t!C (e,g., <br />Pcarson and Swar;;enki. 1<)74) wt"rt' not u-.ed; ratios of <br />thes...' j'i010jkS in lhe potential SOtlft:l'.~ of carbon in Ihe <br />aquifer:-. and rechargt" arca :Ire not known J.nd the infer- <br />ence of theSl' from other information i.... unrdiahle. <br />ReSOtlfl'es wert" unJ\'ailahle for i"otopk-exdl:Jn~e or reac- <br />tion path motlds, and'iO thes...' melhod~ wt"re not u,'iI.:'d. :\ <br />non-~ite-spt:cific l'mpirit:ally-deri\"ed dilution quollcnt <br />equal [0 OB; of the inilial ~roundwat...'r sample acti\'ity was <br />used IU correct the HC ani\'i!ies 1 Vogel, 19-0). while lhis <br />corre...1ion does not physkally reprt".~l'nt He dilution in the <br />aquifers, other n~~earch indicatt's that Jifft"rcncl:'" betwel..'n <br />thb ~impll..', empirical correuion :llld more sophisticlll"<.i <br />approaches are not si!o!nilk':lllt in the lower Tertia!"}' <br />;lquifl:'r~ of the ~;In JU,1O Basin (Phillips l'[ aI., 19H9l, a <br />hytlrogeologlc and hydroch...'mical selling "lmil:tr to the <br />Ar:Jp:.lhOl' and Den\"(:r aquifers <br /> <br />163 <br /> <br />The Roc~~ \Iounl:un A"""OJhon "r G""loJ.:,>I, <br />