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<br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br /> <br />IV. EXPERIMENTAL DESIGN <br /> <br />4.1 Laboratory Experiments <br /> <br />Development of the laboratory experimental design was in itself a <br /> <br />primary goal and an obstacle for this research program. These types of <br /> <br />studies had never been performed before. The ideal design is described <br /> <br />along with the actual procedures used here, as they were compromised by <br /> <br />the limitations of available physical facilities and time. Ice <br /> <br /> <br />nucleation is quantified in the framework of well founded macroscopic <br /> <br /> <br />conceptual models of the various processes that can lead to ice <br /> <br />formation. Standard definitions of these have been given in Chapter 2. <br /> <br />Again, it is important to note that this is not a study of the nature <br /> <br />of the different mechanisms, only of their consequences. The <br /> <br />microscopic details related to each mechanism are not well known, but <br /> <br />are not important for this study. The macroscopic details are important <br /> <br /> <br />because they help define the experiments necessary to isolate the <br /> <br />contributions of different modes for different atmospheric conditions. <br /> <br /> <br />In this regard, the working definitions of the nucleation modes differ <br /> <br />slightly from the standard definitions, and from the definitions given <br /> <br />by DeMott et al. (1983). For example, any nucleation occurring below <br /> <br />water saturation is included as deposition nucleation, since the role <br /> <br />of liquid condensation cannot be discerned. The current definitions are <br />