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<br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br /> <br />41 <br /> <br />this study fractions active were determined with the aid of the <br /> <br />condensation nucleus counter, considered to give an estimate of total <br /> <br /><Aitken) particles. This is discussed further in the following section. <br /> <br />3.3 Aerosol Generation <br /> <br />Cloud condensation and ice nuclei for experimentation are <br /> <br />generated outside the dynamic cloud chamber and can be injected at any <br /> <br />point prior to or during an expansion. A small fan is used to induce <br /> <br />mixing. Po1ydisperse or nearly monodisperse CCN particles of various <br /> <br />compositions can be generated from aqueous solution using a bubbler <br /> <br />system. These solution droplets are dried in a diffusion type drier <br /> <br />before input directly into the chamber or into a Thermo Systems <br /> <br />Incorporated (TSI) Electrostatic Classifier (Model 307l). Particle <br />concentrations in the DCC prior to injection are typically controlled <br /> <br />to be < 0.1 cm-3. The activity of the CCN aerosols used are relatively <br /> <br /> <br />well behaved and can be predicted theoretically (Fitzgerald, 1975). CCN <br /> <br /> <br />concentration can be adjusted over the range 10 to 104 cm-3. Total <br /> <br /> <br />condensation nucleus concentration was not monitored in every <br /> <br />experiment; rather, equivalent timed injections were used for this <br /> <br />study, based on measurements of bubbler output usinga TSI Condensation <br /> <br />Nucleus Counter (Model 3020). <br />Ice nucleating aerosols were generated in a repeatable manner by <br /> <br />solution combustion within a large vertical dilution tunnel. Samples of <br /> <br />ice nuclei were taken directly from the tunnel just before injection <br /> <br />time and were stored in flexibe, electrically conductive bags <br /> <br />(Velostat). When po1ydisperse aerosols were to be injected, this <br /> <br />required dilution with -30oC dewpoint air, due to the high <br />