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<br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br /> <br />15 <br /> <br />supersaturation with respect to water, and the other, at water <br /> <br />saturation, is much slower (minutes). DeMott et al. (1983) had <br /> <br />previously distinguished these potential mechanisms as condensation to <br /> <br /> <br />aqueous embryos followed by freezing, and condensation to droplets <br /> <br />followed by freezing. <br />A method for generating more efficient condensation-freezing ice <br /> <br />nuclei (AgI-AgC1-xNaCl) has been described by Feng and Finnegan (1985; <br /> <br />1989) and has come into use in the operational weather modification <br /> <br /> <br />community over the past few years. Results of experiments in the <br /> <br />dynamic cloud chamber (DeMott, 1988) show that the activity of a <br /> <br />po1ydisperse aerosol of this composition is insensitive to large <br /> <br />changes in ambient droplet concentrations for equivalent injections <br /> <br />into expansion-formed clouds; i.e., the nuclei function predominately <br /> <br />by condensation-freezing or at least form cloudjhaze drops before <br /> <br />droplet-nuclei contact has time to occur. Below water saturation, Feng <br /> <br />et a1. (1989) found these aerosols to be several times to 10 times as <br /> <br />efficient in apparently nucleating ice by deposition, compared to AgI- <br /> <br />AgC1 aerosols. <br /> <br />Preliminary experiments in the CSU dynamic cloud chamber have <br /> <br />also suggested that nuclei aerosol injection prior to warm cloud <br /> <br />condensation influences both the mode and rate of formation of ice by <br /> <br /> <br />AgI-AgCl aerosols (DeMott et a1., 1984a). AgI-AgCl-4NaCl aerosols <br /> <br /> <br />showed no apparent sensitivity to their time history in cloudy air. <br /> <br />2.2 Descriptions of Ice Nuclei Behavior in Cloud Models <br /> <br />Nucleation mechanisms, rates and effectivities can directly and <br /> <br />indirectly influence the nature of numerical cloud model results. Lamb <br />