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<br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br />I <br /> <br />7 <br /> <br />since this is an accepted terminology. It should be quite clear, <br /> <br />however, that this terminology truly refers to the macroscopic process <br /> <br />(sometimes multi-stage) by which an ice crystal forms, and not the <br /> <br />microscopic mechanism that describes how the ice phase first appears or <br /> <br />is ordered on a particle surface. Experiments were designed to <br /> <br />systematically isolate nucleation mechanisms operative by direct <br /> <br />measurement and subtraction methods, primarily using continuous <br /> <br />expansions experiments. For the two nucleants employed, certain <br /> <br />nucleation mechanisms are favored or dominant under some cloud <br /> <br />conditions because of chemical and physical properties and the history <br /> <br />of environmental exposure. Flexibility was inherent in the approach, <br /> <br />but not in the basic framework. <br /> <br />In all experiments, the ice nucleating aerosol, generated in the <br /> <br />same way as in operational weather modification projects, was sampled <br /> <br />and diluted as needed with dry air before injection into the DCC. Two <br /> <br /> <br />types of seeding materials were used. These were AgI-AgCl and AgI-AgCl- <br /> <br /> <br />NaC1 aerosols. These aerosols represent the most efficient AgI-type <br /> <br /> <br />aerosols actively used for weather modification, based on current <br /> <br />knowledge. Most experiments utilized narrow size cuts of particles, in <br /> <br />order to differentiate particle size effects. When such nearly <br /> <br />monodisperse nuclei were desired, the sample was first transferred to a <br /> <br />particle size classifier. The aerosols were injected directly into the <br /> <br />DCC before or after cloud formation, depending on the desired <br /> <br />measurement conditions. Total aerosol concentrations were measured <br /> <br />beforehand. Two particle sizes were generated for the experiments: <br /> <br />distributions of particles closely centered at O. 03 ~m and O. 07 ~m <br /> <br />diameter. This covered a sufficient range of dry particle mobility and <br />